Hochschule für Technik und Umwelt FHNW
Dauerhafte URI für den Bereichhttps://irf.fhnw.ch/handle/11654/35
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Publikation Long‐term trend analysis of aerosol variables at the high‐alpine site Jungfraujoch(Wiley, 13.07.2007) Collaud Coen, Martine; Weingartner, Ernest; Nyeki, Stephan; Cozic, Julie; Henning, Silvia; Verheggen, Bart; Gehrig, Robert; Baltensperger, UrsThis study reports the first long-term trend analysis of aerosol optical measurements at the high-alpine site Jungfraujoch, which started 10.5 years ago. Since the aerosol variables are approximately lognormally distributed, the seasonal Kendall test and Sen's slope estimator were applied as nonparametric methods to detect the long-term trends for each month. The yearly trend was estimated by a least-mean-square fit, and the number of years necessary to detect this trend was calculated. The most significant trend is the increase (4–7% yr−1) in light-scattering coefficients during the September to December period. The light absorption and backscattering coefficients and the aerosol number concentration also show a positive trend during this time of the year. The hemispheric backscattering fraction and the scattering exponent calculated with the smaller wavelengths (450 and 550 nm), which relate to the small aerosol size fraction, decrease except during the summer, whereas the scattering exponent calculated with the larger wavelengths (550 and 700 nm) remains constant. Generally, the summer months at the Jungfraujoch, which are strongly influenced by planetary boundary layer air masses, do not show any long-term trend. The trends determined by least-mean-square fits of the scattering and backscattering coefficients, the hemispheric backscattering fractions, and the scattering exponent are significant, and the number of years necessary to detect them is shorter than 10 years. For these variables, the trends and the slopes estimated by the seasonal Kendall test are therefore confirmed by the least-mean-square fit results.01A - Beitrag in wissenschaftlicher ZeitschriftPublikation Climatology of aerosol radiative properties in the free troposphere(Elsevier, 04.12.2011) Andrews, Elisabeth; Ogren, John A.; Bonasoni, Paolo; Marinoni, Angela; Cuevas, Emilio; Rodríguez, Sergio Hugo Sánchez; Sun, Junying; Jaffe, Daniel A.; Fischer, Emily V.; Baltensperger, Urs; Weingartner, Ernest; Collaud Coen, Martine; Sharma, Sangeeta; Macdonald, Annemarie; Leaitch, W. Richard; Lin, Neng Huei; Laj, Paolo; Arsov, Todor; Kalapov, Ivo; Jefferson, Anne; Sheridan, Patrick01A - Beitrag in wissenschaftlicher ZeitschriftPublikation Analysis of long‐term aerosol size distribution data from Jungfraujoch with emphasis on free tropospheric conditions, cloud influence, and air mass transport(Wiley, 2015) Herrmann, Erik; Weingartner, Ernest; Henne, Stephan; Vuilleumier, Laurent; Bukowiecki, Nicolas; Steinbacher, Martin; Conen, Franz; Collaud Coen, Martine; Hammer, Emanuel; Jurányi, Zsófia; Baltensperger, Urs; Gysel, MartinSix years of aerosol size distribution measurements between 20 and 600 nm diameters and total aerosol concentration above 10 nm from March 2008 to February 2014 at the high‐alpine site Jungfraujoch are presented. The size distribution was found to be typically bimodal with mode diameters and widths relatively stable throughout the year and the observation period. New particle formation was observed on 14.5% of all days without a seasonal preference. Particles typically grew only into the Aitken mode and did not reach cloud condensation nucleus (CCN) sizes on the time scale of several days. Growth of preexisting particles in the Aitken mode, on average, contributed very few CCN. We concluded that the dominant fraction of CCN at Jungfraujoch originated in the boundary layer. A number of approaches were used to distinguish free tropospheric (FT) conditions and episodes with planetary boundary layer (PBL) influence. In the absence of PBL injections, the concentration of particles larger than 90 nm (N90, roughly corresponding to the CCN concentration) reached a value ~40 cm−3 while PBL influence caused N90 concentrations of several hundred or even 1000 cm−3. Comparing three criteria for free tropospheric conditions, we found FT prevalence for 39% of the time with over 60% during winter and below 20% during summer. It is noteworthy that a simple criterion based on standard trace gas measurements appeared to outperform alternative approaches.01A - Beitrag in wissenschaftlicher Zeitschrift