Effects of relative humidity on aerosol light scattering. results from different European sites
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Autor:innen
Autor:in (Körperschaft)
Publikationsdatum
2013
Typ der Arbeit
Studiengang
Typ
01A - Beitrag in wissenschaftlicher Zeitschrift
Herausgeber:innen
Herausgeber:in (Körperschaft)
Betreuer:in
Übergeordnetes Werk
Atmospheric Chemistry and Physics
Themenheft
DOI der Originalpublikation
Link
Reihe / Serie
Reihennummer
Jahrgang / Band
13
Ausgabe / Nummer
21
Seiten / Dauer
10609–10631
Patentnummer
Verlag / Herausgebende Institution
Copernicus
Verlagsort / Veranstaltungsort
Göttingen
Auflage
Version
Programmiersprache
Abtretungsempfänger:in
Praxispartner:in/Auftraggeber:in
Zusammenfassung
The effect of aerosol water uptake on the aerosol particle light scattering coefficient (σsp) is described in this study by comparing measurements from five European sites: the Jungfraujoch, located in the Swiss Alps at 3580 m a.s.l.; Ny-Ålesund, located on Spitsbergen in the Arctic; Mace Head, a coastal site in Ireland; Cabauw, a rural site in the Netherlands; and Melpitz, a regional background site in Eastern Germany. These sites were selected according to the aerosol type usually encountered at that location. The scattering enhancement factor f(RH, λ) is the key parameter to describe the effect of water uptake on the particle light scattering. It is defined as the σsp(RH) at a certain relative humidity (RH) and wavelength λ divided by its dry value. f(RH) at the five sites varied widely, starting at very low values of f(RH = 85%, λ = 550 nm) around 1.28 for mineral dust, and reaching up to 3.41 for Arctic aerosol. Hysteresis behavior was observed at all sites except at the Jungfraujoch (due to the absence of sea salt). Closure studies and Mie simulations showed that both size and chemical composition determine the magnitude of f(RH). Both parameters are also needed to successfully predict f(RH). Finally, the measurement results were compared to the widely used aerosol model, OPAC (Hess et al., 1998). Significant discrepancies were seen, especially at intermediate RH ranges; these were mainly attributed to inappropriate implementation of hygroscopic growth in the OPAC model. Replacement of the hygroscopic growth with values from the recent literature resulted in a clear improvement of the OPAC model.
Schlagwörter
Fachgebiet (DDC)
550 - Geowissenschaften
Veranstaltung
Startdatum der Ausstellung
Enddatum der Ausstellung
Startdatum der Konferenz
Enddatum der Konferenz
Datum der letzten Prüfung
ISBN
ISSN
1680-7324
1680-7316
1680-7316
Sprache
Englisch
Während FHNW Zugehörigkeit erstellt
Nein
Publikationsstatus
Veröffentlicht
Begutachtung
Peer-Review der ganzen Publikation
Open Access-Status
Gold
Lizenz
Zitation
ZIEGER, Paul, Rahel FIERZ-SCHMIDHAUSER, Ernest WEINGARTNER und Urs BALTENSPERGER, 2013. Effects of relative humidity on aerosol light scattering. results from different European sites. Atmospheric Chemistry and Physics. 2013. Bd. 13, Nr. 21, S. 10609–10631. DOI 10.5194/acp-13-10609-2013. Verfügbar unter: https://doi.org/10.26041/fhnw-8173