Seasonal and diurnal characteristics of water soluble inorganic compounds in the gas and aerosol phase in the Zurich area
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Autor:innen
Fisseha, Rebeka
Dommen, Josef
Gutzwiller, Lukas
Gysel, Martin
Emmenegger, C.
Kalberer, Markus
Baltensperger, Urs
Autor:in (Körperschaft)
Publikationsdatum
2006
Typ der Arbeit
Studiengang
Typ
01A - Beitrag in wissenschaftlicher Zeitschrift
Herausgeber:innen
Herausgeber:in (Körperschaft)
Betreuer:in
Übergeordnetes Werk
Atmospheric Chemistry and Physics
Themenheft
DOI der Originalpublikation
Link
Reihe / Serie
Reihennummer
Jahrgang / Band
6
Ausgabe / Nummer
7
Seiten / Dauer
1895-1904
Patentnummer
Verlag / Herausgebende Institution
Copernicus
Verlagsort / Veranstaltungsort
Göttingen
Auflage
Version
Programmiersprache
Abtretungsempfänger:in
Praxispartner:in/Auftraggeber:in
Zusammenfassung
Gas and aerosol samples were taken using a wet effluent diffusion denuder/aerosol collector (WEDD/AC) coupled to ion chromatography (IC) in the city of Zurich, Switzerland from August to September 2002 and in March 2003. Major water soluble inorganic ions; nitrate, sulfate, and nitrite were analyzed online with a time resolution of two hours for the gas and aerosol phase. The fraction of water soluble inorganic anions in PM10 varied from 15% in August to about 38% in March. Seasonal and diurnal variations of nitrate in the gas and aerosol phase were observed with more than 50% of the total nitrate in the gas phase during August and more than 80% of nitrate in the aerosol phase during March exceeding the concentration of sulfate by a factor of 2. Aerosol sulfate, on the other hand, did not show significant variability with season. However, in the gas phase, the SO2 concentration was 6.5 times higher in winter than in summer. Nitrous acid (HONO) also showed a diurnal variation in both the gas and aerosol phase with the lowest concentration (0.2–0.6 µg/m³) in the afternoon. The primary pollutants, NO, CO and SO2 mixing ratios were often at their highest between 04:00–10:00 local time due to the build up of fresh vehicle emission under a nocturnal inversion.
Schlagwörter
Fachgebiet (DDC)
660 - Technische Chemie
Veranstaltung
Startdatum der Ausstellung
Enddatum der Ausstellung
Startdatum der Konferenz
Enddatum der Konferenz
Datum der letzten Prüfung
ISBN
ISSN
1680-7324
1680-7316
1680-7316
Sprache
Englisch
Während FHNW Zugehörigkeit erstellt
Nein
Publikationsstatus
Veröffentlicht
Begutachtung
Peer-Review der ganzen Publikation
Open Access-Status
Gold
Lizenz
Zitation
FISSEHA, Rebeka, Josef DOMMEN, Lukas GUTZWILLER, Ernest WEINGARTNER, Martin GYSEL, C. EMMENEGGER, Markus KALBERER und Urs BALTENSPERGER, 2006. Seasonal and diurnal characteristics of water soluble inorganic compounds in the gas and aerosol phase in the Zurich area. Atmospheric Chemistry and Physics. 2006. Bd. 6, Nr. 7, S. 1895–1904. DOI 10.5194/acp-6-1895-2006. Verfügbar unter: https://doi.org/10.26041/fhnw-9794