Summertime NOy speciation at the Jungfraujoch, 3580 m above sea level, Switzerland
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Autor:innen
Zellweger, Christoph
Ammann, Markus
Buchmann, Brigitte
Hofer, Patrick
Lugauer, Matthias
Rüttimann, Ralph
Streit, Niklaus
Baltensperger, Urs
Autor:in (Körperschaft)
Publikationsdatum
16.03.2000
Typ der Arbeit
Studiengang
Typ
01A - Beitrag in wissenschaftlicher Zeitschrift
Herausgeber:innen
Herausgeber:in (Körperschaft)
Betreuer:in
Übergeordnetes Werk
Journal of Geophysical Research: Atmospheres
Themenheft
DOI der Originalpublikation
Link
Reihe / Serie
Reihennummer
Jahrgang / Band
105
Ausgabe / Nummer
D5
Seiten / Dauer
6655-6667
Patentnummer
Verlag / Herausgebende Institution
Wiley
Verlagsort / Veranstaltungsort
Hoboken
Auflage
Version
Programmiersprache
Abtretungsempfänger:in
Praxispartner:in/Auftraggeber:in
Zusammenfassung
During summer 1997, speciated reactive nitrogen (NO, NO2, peroxyacetyl nitrate (PAN), HNO3, and particulate nitrate) was measured in conjunction with total reactive nitrogen (NOy) at the high-alpine research station Jungfraujoch (JFJ), 3580 m above sea level (asl). The individually measured NOy components averaged to 82% of total NOy. PAN was the most abundant reactive nitrogen compound and composed on average 36% of NOy, followed by NOx, (22%), particulate nitrate (17%), and HNO3 (7%). The NOx/NOy ratio averaged 0.25, but significantly lower values (0.15–0.20) were observed in the presence of high NOy mixing ratios. A classification of the data by synoptic weather conditions indicated that thermally driven vertical transport has a strong impact on the mixing ratios measured at the JFJ during summer. A strong diurnal cycle with maximum mixing ratios in the late afternoon was observed for convective days with north-westerly advection at 500 hPa. In contrast, during a period of convective days with a wind speed below 7.5 m/s at 500 hPa, no obvious diurnal cycle was observed. Under these meteorological conditions the convective boundary layer can be significantly higher over the Alps (i.e., around 4 km asl) than over the surrounding lowlands. Subsequent advection may finally result in the export of reactive nitrogen reservoir compounds to the free troposphere and hence influence global atmospheric chemistry.
Schlagwörter
Fachgebiet (DDC)
550 - Geowissenschaften
570 - Biowissenschaften, Biologie
570 - Biowissenschaften, Biologie
Veranstaltung
Startdatum der Ausstellung
Enddatum der Ausstellung
Startdatum der Konferenz
Enddatum der Konferenz
Datum der letzten Prüfung
ISBN
ISSN
2169-897X
2169-8996
2169-8996
Sprache
Englisch
Während FHNW Zugehörigkeit erstellt
Nein
Zukunftsfelder FHNW
Publikationsstatus
Veröffentlicht
Begutachtung
Peer-Review der ganzen Publikation
Open Access-Status
Closed
Lizenz
Zitation
ZELLWEGER, Christoph, Markus AMMANN, Brigitte BUCHMANN, Patrick HOFER, Matthias LUGAUER, Ralph RÜTTIMANN, Niklaus STREIT, Ernest WEINGARTNER und Urs BALTENSPERGER, 2000. Summertime NOy speciation at the Jungfraujoch, 3580 m above sea level, Switzerland. Journal of Geophysical Research: Atmospheres. 16 März 2000. Bd. 105, Nr. D5, S. 6655–6667. DOI 10.1029/1999jd901126. Verfügbar unter: https://irf.fhnw.ch/handle/11654/46894