Comparing black carbon and aerosol absorption measuring instruments – a new system using lab-generated soot coated with controlled amounts of secondary organic matter

We report on an inter-comparison of black-carbon- and aerosol-absorption-measuring instruments with laboratory-generated soot particles coated with controlled amounts of secondary organic matter (SOM). The aerosol generation setup consisted of a miniCAST 5201 Type BC burner for the generation of soot particles and a new automated oxidation flow reactor based on the micro smog chamber (MSC) for the generation of SOM from the ozonolysis of α-pinene. A series of test aerosols was generated with elemental to total carbon (EC / TC) mass fraction ranging from about 90 % down to 10 % and single-scattering albedo (SSA at 637 nm) from almost 0 to about 0.7. A dual-spot Aethalometer AE33, a photoacoustic extinctiometer (PAX, 870 nm), a multi-angle absorption photometer (MAAP), a prototype photoacoustic instrument, and two prototype photo-thermal interferometers (PTAAM-2λ and MSPTI) were exposed to the test aerosols in parallel. Significant deviations in the response of the instruments were observed depending on the amount of secondary organic coating. We believe that the setup and methodology described in this study can easily be standardised and provide a straightforward and reproducible procedure for the inter-comparison and characterisation of both filter-based and in situ black-carbon-measuring (BC-measuring) instruments based on realistic test aerosols.

Schlagwörter

Fachgebiet (DDC)

620 - Ingenieurwissenschaften und Maschinenbau

Projekt

Veranstaltung

Startdatum der Ausstellung

Enddatum der Ausstellung

Startdatum der Konferenz

Enddatum der Konferenz

Datum der letzten Prüfung

ISBN

ISSN

1867-8548

Sprache

Englisch

Während FHNW Zugehörigkeit erstellt

Ja

Zukunftsfelder FHNW

Publikationsstatus

Veröffentlicht

Begutachtung

Peer-Review der ganzen Publikation

Open Access-Status

Gold

Lizenz

Zitation

KALBERMATTER, Daniel M., Griša MOČNIK, Luka DRINOVEC, Bradley VISSER, Jannis RÖHRBEIN, Matthias OSCITY, Ernest WEINGARTNER, Antti-Pekka HYVÄRINEN und Konstantina VASILATOU, 2022. Comparing black carbon and aerosol absorption measuring instruments – a new system using lab-generated soot coated with controlled amounts of secondary organic matter. Atmospheric Measurement Techniques. 2022. Bd. 15, Nr. 2, S. 561–572. DOI 10.5194/amt-15-561-2022. Verfügbar unter: https://doi.org/10.26041/fhnw-7613

Komplettanzeige