Hygroscopic properties of submicrometer atmospheric aerosol particles measured with H-TDMA instruments in various environments - a review

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Authors
Swietlicki, Erik
Hansson, Hans-Christen
Hämeri, Kaarle
Svenningsson, Birgitta
Massling, Andreas
McFiggans, Gordon
McMurry, Peter H.
Petäjä, Tuukka
Tunved, Peter
Author (Corporation)
Publication date
01.01.2008
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Type
01A - Journal article
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Editor (Corporation)
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Parent work
Tellus B: Chemical and Physical Meteorology
Special issue
Link
Series
Series number
Volume
60
Issue / Number
3
Pages / Duration
432-469
Patent number
Publisher / Publishing institution
Stockholm University Press
Place of publication / Event location
Stockholm
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Abstract
The hygroscopic properties play a vital role for the direct and indirect effects of aerosols on climate, as well as the health effects of particulate matter (PM) by modifying the deposition pattern of inhaled particles in the humid human respiratory tract. Hygroscopic Tandem Differential Mobility Analyzer (H-TDMA) instruments have been used in field campaigns in various environments globally over the last 25 yr to determine the water uptake on submicrometre particles at subsaturated conditions. These investigations have yielded valuable and comprehensive information regarding the particle hygroscopic properties of the atmospheric aerosol, including state of mixing. These properties determine the equilibrium particle size at ambient relative humidities and have successfully been used to calculate the activation of particles at water vapour supersaturation. This paper summarizes the existing published H-TDMA results on the sizeresolved submicrometre aerosol particle hygroscopic properties obtained from ground-based measurements at multiple marine, rural, urban and free tropospheric measurement sites. The data is classified into groups of hygroscopic growth indicating the external mixture, and providing clues to the sources and processes controlling the aerosol. An evaluation is given on how different chemical and physical properties affect the hygroscopic growth.
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Subject (DDC)
550 - Geowissenschaften
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ISBN
ISSN
1600-0889
0280-6509
Language
English
Created during FHNW affiliation
No
Strategic action fields FHNW
Publication status
Published
Review
Peer review of the complete publication
Open access category
Gold
License
'https://creativecommons.org/licenses/by/4.0/'
Citation
SWIETLICKI, Erik, Hans-Christen HANSSON, Kaarle HÄMERI, Birgitta SVENNINGSSON, Andreas MASSLING, Gordon MCFIGGANS, Peter H. MCMURRY, Tuukka PETÄJÄ, Peter TUNVED, Martin GYSEL, David TOPPING, Ernest WEINGARTNER, Urs BALTENSPERGER, Jenny RISSLER, Alfred WIEDENSOHLER und Markku KULMALA, 2008. Hygroscopic properties of submicrometer atmospheric aerosol particles measured with H-TDMA instruments in various environments - a review. Tellus B: Chemical and Physical Meteorology. 1 Januar 2008. Bd. 60, Nr. 3, S. 432–469. DOI 10.1111/j.1600-0889.2008.00350.x. Verfügbar unter: https://doi.org/10.26041/fhnw-9744