lnstitut für Sensorik und Elektronik

Dauerhafte URI für die Sammlunghttps://irf.fhnw.ch/handle/11654/28068

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Autor:in: search.filters.author.Nyeki, StephanThema: search.filters.subject.620 - Ingenieurwissenschaften und Maschinenbau

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    Publikation
    Properties of jet engine combustion particles during the PartEmis experiment: Hygroscopicity at subsaturated conditions
    (Wiley, 06.06.2003) Gysel, Martin; Nyeki, Stephan; Weingartner, Ernest; Baltensperger, Urs; Giebl, Heinrich; Hitzenberger, Regina; Petzold, Andreas; Wilson, C. W.
    Hygroscopic properties of combustion particles were measured online with a Hygroscopicity Tandem Differential Mobility Analyzer (H-TDMA) during PartEmis jet engine combustor experiments. The combustor was operated at old and modern cruise conditions with fuel sulfur contents (FSC) of 50, 410 and 1270 μg/g, and hygroscopic growth factors (HGF) of particles with different dry diameters were investigated at relative humidities RH ≤ 95%. HGFs increased strongly with increasing FSC (HGF[95% RH, 50 nm, modern cruise] = 1.01 and 1.16 for low and high FSC, respectively), and decreased with increasing particle size at fixed FSC, whereas no significant difference was detected between old and modern cruise. HGFs agreed well with a two-parameter theoretical model which provided an estimate of the sulfuric acid content of dry particles, indicating a nearly linear dependence on FSC.
    01A - Beitrag in wissenschaftlicher Zeitschrift
  • Kein Vorschaubild vorhanden
    Publikation
    Properties of jet engine combustion particles during the PartEmis experiment. Hygroscopic growth at supersaturated conditions
    (Wiley, 31.07.2003) Hitzenberger, Regina; Giebl, Heinrich; Petzold, Andreas; Gysel, Martin; Nyeki, Stephan; Weingartner, Ernest; Baltensperger, Urs; Wilson, C. W.
    During the EU Project PartEmis, the microphysical properties of aircraft combustion aerosol were investigated. This study is focused on the ability of exhaust aerosols to act as cloud condensation nuclei (CCN). The combustor was operated at two different conditions representing old and modern aircraft engine technology. CCN concentrations were measured with the University of Vienna CCN counter [Giebl et al., 2002] at supersaturations around 0.7%. The activation ratio (fraction of CCN in total aerosol) depended on the fuel sulphur content (FSC) and also on the operation conditions. CCN/CN ratios increased from 0.93 through 1.43 to 5.15*10ˉ³ (old cruise conditions) and 0.67 through 3.04 to 7.94*10ˉ³ (modern cruise conditions) when FSC increased from 50 through 410 to1270 μg/g. The activation behaviour was modelled using classical theories and with a semi-empirical model [Gysel et al., 2003] based on measured hygroscopicity of the aerosol under subsaturated conditions, which gave the best agreement.
    01A - Beitrag in wissenschaftlicher Zeitschrift
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    Publikation
    Separation of volatile and non-volatile aerosol fractions by thermodesorption. instrumental development and applications
    (Elsevier, 04/2001) Burtscher, Heinz; Baltensperger, Urs; Bukowiecki, Nicolas; Cohn, P.; Hüglin, Christoph; Mohr, Martin; Matter, Urs; Nyeki, Stephan; Schmatloch, Volker; Streit, Niklaus; Weingartner, Ernest
    An instrument to remove volatile material from aerosol particles by thermal desorption is presented. The thermodesorber consists of a heated tube, where volatile material is desorbed from the particles, and a water- or air-cooled tube, consisting of activated charcoal. This last tube removes desorbed material and thus prevents it from re-adsorbing onto particles. Although designed for measuring particulate emissions from combustion processes it can also be applied to atmospheric aerosols. After theoretical and experimental determination of thermodesorber operating characteristics (temperature profile, losses, removal of desorbed material), examples of applications in several fields are given. Examples of atmospheric measurements at several remote and urban sites are presented. In combustion technology, the thermodesorber is applied to remove all volatile materials, allowing separation of volatile species and the non-volatile core (mainly elemental carbon) of combustion particles. Finally, the thermodesorber is used to study adsorption and desorption processes of polycyclic aromatic hydrocarbons on particles.
    01A - Beitrag in wissenschaftlicher Zeitschrift