Surface water treatment by UV/H2O2 with subsequent soil aquifer treatment. Impact on micropollutants, dissolved organic matter and biological activity
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Dateien
Autor:innen
Wünsch, Robin
Plattner, Julia
Cayon, David
Gebhardt, Jens
Wülser, Richard
von Gunten, Urs
Autor:in (Körperschaft)
Publikationsdatum
2019
Typ der Arbeit
Studiengang
Sammlung
Typ
01A - Beitrag in wissenschaftlicher Zeitschrift
Herausgeber:innen
Herausgeber:in (Körperschaft)
Betreuer:in
Übergeordnetes Werk
Environmental Science. Water, Research & Technology
Themenheft
DOI der Originalpublikation
Link
Reihe / Serie
Reihennummer
Jahrgang / Band
5
Ausgabe / Nummer
10
Seiten / Dauer
1709-1722
Patentnummer
Verlag / Herausgebende Institution
Royal Society of Chemistry
Verlagsort / Veranstaltungsort
Auflage
Version
Programmiersprache
Abtretungsempfänger:in
Praxispartner:in/Auftraggeber:in
Zusammenfassung
Because organic micropollutants (MP) are frequently detected in river waters that are used as drinking water sources, combining a relatively cost-efficient natural treatment with upstream advanced oxidation processes (AOP) appears promising for their efficient abatement. Such a multi-barrier system can be integrated in drinking water production schemes to minimize risks from potentially hazardous MPs. This study investigates the impact of an UV/H2O2 AOP before soil aquifer treatment (SAT) on the abatement of selected MPs (EDTA, acesulfame, iopamidol, iomeprol, metformin, 1H-benzotriazole, iopromide), dissolved organic matter (DOM) (apparent molecular size distribution, specific UV absorbance at 254 nm – SUVA) and microbial parameters (intact cell count, cell-bound ATP). A pilot plant consisting of an AOP (0.5 m3 h−1, 4 mg L−1 H2O2, 6000 J m−2) and two parallel soil columns (filtration velocity: 1 m d−1, column height: 1 m) was continuously operated over a period of 15 months with Rhine river water pre-treated with rapid sand filtration. The investigations revealed a shift towards longer retention times of the humic substances peak in LC analysis of DOM, lower SUVA and higher biodegradability of DOM after UV/H2O2 treatment. In addition, an overall higher abatement of all investigated MPs by the combined treatment was observed (AOP with subsequent SAT) compared to either process alone. This observation could be explained by an addition of the single treatment effects. The strong primary disinfection effect of the AOP was detectable along the first meter of infiltration, but did not lead to any change in the column performance (i.e., similar abatement of dissolved organic matter).
Schlagwörter
Micropollutants, Drinking water
Fachgebiet (DDC)
540 - Chemie
Veranstaltung
Startdatum der Ausstellung
Enddatum der Ausstellung
Startdatum der Konferenz
Enddatum der Konferenz
Datum der letzten Prüfung
ISBN
ISSN
2053-1400
2053-1419
2053-1419
Sprache
Englisch
Während FHNW Zugehörigkeit erstellt
Ja
Publikationsstatus
Veröffentlicht
Begutachtung
Peer-Review der ganzen Publikation
Open Access-Status
Hybrid
Lizenz
Zitation
WÜNSCH, Robin, Julia PLATTNER, David CAYON, Fabienne EUGSTER, Jens GEBHARDT, Richard WÜLSER, Urs VON GUNTEN und Thomas WINTGENS, 2019. Surface water treatment by UV/H2O2 with subsequent soil aquifer treatment. Impact on micropollutants, dissolved organic matter and biological activity. Environmental Science. Water, Research & Technology. 2019. Bd. 5, Nr. 10, S. 1709–1722. DOI 10.1039/C9EW00547A. Verfügbar unter: https://doi.org/10.26041/fhnw-4162