EUCAARI ion spectrometer measurements at 12 European sites – analysis of new particle formation events

We present comprehensive results on continuous atmospheric cluster and particle measurements in the size range ~1–42 nm within the European Integrated project on Aerosol Cloud Climate and Air Quality interactions (EUCAARI) project. We focused on characterizing the spatial and temporal variation of new particle formation events and relevant particle formation parameters across Europe. Different types of air ion and cluster mobility spectrometers were deployed at 12 field sites across Europe from March 2008 to May 2009. The measurements were conducted in a wide variety of environments, including coastal and continental locations as well as sites at different altitudes (both in the boundary layer and the free troposphere). New particle formation events were detected at all of the 12 field sites during the year-long measurement period. From the data, nucleation and growth rates of newly formed particles were determined for each environment. In a case of parallel ion and neutral cluster measurements, we could also estimate the relative contribution of ion-induced and neutral nucleation to the total particle formation. The formation rates of charged particles at 2 nm accounted for 1–30% of the corresponding total particle formation rates. As a significant new result, we found out that the total particle formation rate varied much more between the different sites than the formation rate of charged particles. This work presents, so far, the most comprehensive effort to experimentally characterize nucleation and growth of atmospheric molecular clusters and nanoparticles at ground-based observation sites on a continental scale.

Schlagwörter

Fachgebiet (DDC)

550 - Geowissenschaften

Projekt

Veranstaltung

Startdatum der Ausstellung

Enddatum der Ausstellung

Startdatum der Konferenz

Enddatum der Konferenz

Datum der letzten Prüfung

ISBN

ISSN

1680-7324
1680-7316

Sprache

Englisch

Während FHNW Zugehörigkeit erstellt

Nein

Publikationsstatus

Veröffentlicht

Begutachtung

Peer-Review der ganzen Publikation

Open Access-Status

Gold

Lizenz

Zitation

MANNINEN, Hanna E., Tuomo NIEMINEN, Eija ASMI, Stéphanie GAGNÉ, Silja HÄKKINEN, Katrianne LEHTIPALO, Pasi Pekka AALTO, Marko VANA, Aadu MIRME, Sander MIRME, Urmas HÕRRAK, Christian PLASS-DÜLMER, Gert STANGE, Gyula KISS, András HOFFER, N. TÖRŐ, Marcel MOERMAN, Bas HENZING, Gerrit DE LEEUW, Marcel BRINKENBERG, Giorgos N. KOUVARAKIS, Aikaterini BOUGIATIOTI, Nikolaos MIHALOPOULOS, Colin D. O’DOWD, Darius CEBURNIS, Almut ARNETH, Brigitta SVENNINGSSON, Erik SWIETLICKI, Leone TAROZZI, Stefano DECESARI, Maria Cristina FACCHINI, Wolfram BIRMILI, André SONNTAG, Alfred WIEDENSOHLER, Julien BOULON, Karine SELLEGRI, Paolo LAJ, Martin GYSEL, Nicolas BUKOWIECKI, Ernest WEINGARTNER, Günther WEHRLE, Ari LAAKSONEN, Amar HAMED, Jorma JOUTSENSAARI, Tuukka PETÄJÄ, Veli-Matti KERMINEN und Markku KULMALA, 2010. EUCAARI ion spectrometer measurements at 12 European sites – analysis of new particle formation events. Atmospheric Chemistry and Physics. 25 August 2010. Bd. 10, Nr. 16, S. 7907–7927. DOI 10.5194/acp-10-7907-2010. Verfügbar unter: https://doi.org/10.26041/fhnw-9667

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