lnstitut für Sensorik und Elektronik
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Publikation A European aerosol phenomenology - 1. physical characteristics of particulate matter at kerbside, urban, rural and background sites in Europe(Elsevier, 05/2004) Van Dingenen, Rita; Raes, Frank; Putaud, Jean-Philippe; Baltensperger, Urs; Charron, Aurélie; Facchini, Maria Cristina; Decesari, Stefano; Fuzzi, Sandro; Gehrig, Robert; Hansson, Hans-Christen; Harrison, Roy M.; Hüglin, Cristoph; Jones, Alan M.; Laj, Paolo; Lorbeer, Gundi; Maenhaut, Willy; Palmgren, Finn; Querol, Xavier; Rodriguez, Sergio; Schneider, Jürgen; ten Brink, Harry; Tunved, Peter; Tørseth, Kjetil; Wehner, Birgit; Weingartner, Ernest; Wiedensohler, Alfred; Wåhlin, PeterThis paper synthesizes data on aerosol (particulate matter, PM) physical characteristics, which were obtained in European aerosol research activities at free-troposphere, natural, rural, near-city, urban, and kerbside sites over the past decade. It covers only two sites in the semi-arid Mediterranean area, and lacks data from Eastern Europe. The data include PM10 and/or PM2.5 mass concentrations, and aerosol particle size distributions. Such data sets are more comprehensive than those currently provided by air quality monitoring networks (e.g. EMEP, EUROAIRNET). Data available from 31 sites in Europe (called “The Network”) were reviewed. They were processed and plotted to allow comparisons in spite of differences in the sampling and analytical techniques used in various studies. A number of conclusions are drawn as follows: Background annual average PM10 and PM2.5 mass concentrations for continental Europe are 7.0±4.1 and 4.8±2.4 μg mˉ³, respectively. The EU 2005 annual average PM10 standard of 40 μg mˉ³ is exceeded at a few sites in The Network. At all near city, urban and kerbside sites, the EU 2010 annual average PM10 standard of 20 μg mˉ³, as well as the US-EPA annual average PM2.5 standard of 15 μg mˉ³ are exceeded. In certain regions, PM10 and PM2.5 in cities are strongly affected by the regional aerosol background. There is no “universal” (i.e. valid for all sites) ratio between PM2.5 and PM10 mass concentrations, although fairly constant ratios do exist at individual sites. There is no universal correlation between PM mass concentration on the one hand, and total particle number concentration on the other hand, although a ‘baseline’ ratio between number and mass is found for sites not affected by local emissions. This paper is the first part of two companion papers of which the second part describes chemical characteristics.01A - Beitrag in wissenschaftlicher ZeitschriftPublikation Vertical distribution of aerosol particles and NOx close to a motorway(Elsevier, 10/2005) Imhof, D.; Weingartner, Ernest; Vogt, Ulrich; Dreiseidler, Anja; Rosenbohm, E.; Scheer, Volker; Vogt, Rainer; Nielsen, Ole John; Kurtenbach, Ralf; Corsmeier, Ulrich; Kohler, M.; Baltensperger, UrsIn May 2001, the large-scale field project BAB II was performed at the highly frequented motorway BAB (Bundesautobahn) A656 with two traffic lanes in each direction between the German cities Heidelberg and Mannheim. Extensive measurements of air pollutants were carried out on both sides of the motorway. In a distance of 60 m (north side) and 84 m (south side) to the traffic lanes, two 52-m-high towers were installed, at which electrically powered elevators were fixed. In these elevators, two NOx analysers, an Electrical Low Pressure Impactor (ELPI; measurement of the particle number size distribution in the diameter range 𝐷 between 30 nm and 10 μm) and a Diffusion Charger (DC; measuring the particle surface area concentration), were operated to record continuous vertical profiles from 5 to 50 m above the earth's surface. On the upwind side, particle number and surface area concentration as well as NOx values were constant over the entire height profile. On the downwind side, increased concentrations appeared in the near-ground range: in the forenoon, a monotonous decrease in pollutant concentrations with increasing height was found, while around noon the concentration maximum of the particles was slightly shifted to 10 m above ground. This height dependence was found for two different size ranges, i.e., for particles with 𝐷<300nm (consisting of soot particles and nucleation mode particles formed by condensation as a result of cooling of the exhaust gas after emission), and for coarse particles (𝐷>1μm, abrasion and resuspension products). In the size range between 300 and 700 nm, no height dependence was found, corroborating the fact that motor traffic emits only few particles in this size range. On the downwind side of the motorway, only background concentrations were measured above 25 m. The results of the profile measurements were confirmed by stationary measurements of particle size distributions with Scanning Mobility Particle Sizers (SMPS) at various heights. A good correlation between particle surface area and NOx concentration was observed. Vehicle emission factors were determined for the particle surface area, number and volume of several size ranges.01A - Beitrag in wissenschaftlicher Zeitschrift